Determination of the wavelength dependence of refractive indices of flame soot

Abstract

The spectral variation of the optical properties of soot particles is determined by combining classical and dynamic light scattering measurements with the Kramers-Krönig relations. Particle size and number densities are determined from scattering/extinction and autocorrelation measurements at the wavelength of 0.488 μm. This information is then combined with the spectral extinction measurements in the wavelength range 0.2 to 6.4 μm to determine the spectral variation of the refractive indices of flame soot. Results are presented for a premixed propane-oxygen flame with a fuel equivalence ratio ϕ = 1.8. The sensitivity of the technique and its advantage over the previous methods are discussed.