«2+1<sub>B</sub>» tricarbonyl complexes of technetium-99<i>m </i>and rhenium with n,n'-bidentate ligands and methyl 2-(decylthio)-6-isocyanohexanoate

Author:

Miroslavov A. E.123,Kuz'min V. V.4,Sakhonenkova A. P.123,Tyupina M. Yu.13,Sidorenko G. V.13,Kochergina A. R.13,Polukeev V. A.4

Affiliation:

1. Khlopin Radium Institute

2. St. Petersburg State University

3. Ozersk Institute of Technology, Branch of National Research Nuclear University MEPhI

4. AO Vekton

Abstract

«2+1B» tricarbonyl complexes of the general formula [M(CO)3(N^N)CN(CH2)4CH(COOMe)SC10H21]ClO4, where M = 99 m Tc or Re, N^N = 2,2'-bipyridine (bipy) or 1,10-phenanthroline (phen), were prepared by the reaction of [M(CO)3(N^N)(MeOH)]ClO4 with methyl 2-(decylthio)-6-isocyanohexanoate in methanol. The rhenium complexes were isolated and characterized by 1H NMR and IR spectroscopy. The formation of technetium-99 m complexes was con rmed by HPLC. The lipophilicity of the technetium complexes was measured.

Publisher

The Russian Academy of Sciences

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