Optical Properties of Conical Quantum Dot: Exciton-Related Raman Scattering, Interband Absorption and Photoluminescence

Author:

Gavalajyan Sargis P.1,Mantashian Grigor A.12ORCID,Kharatyan Gor Ts.1,Sarkisyan Hayk A.1,Mantashyan Paytsar A.12,Baskoutas Sotirios3ORCID,Hayrapetyan David B.12

Affiliation:

1. Department of General Physics and Quantum Nanostructures, Russian-Armenian University, 123 Hovsep Emin Str., Yerevan 0051, Armenia

2. Institute of Chemical Physics after A.B. Nalbandyan of NAS RA, 5/2 Paruyr Sevak St., Yerevan 0014, Armenia

3. Department of Materials Science, University of Patras, 265 04 Patras, Greece

Abstract

The current work used the effective mass approximation conjoined with the finite element method to study the exciton states in a conical GaAs quantum dot. In particular, the dependence of the exciton energy on the geometrical parameters of a conical quantum dot has been studied. Once the one-particle eigenvalue equations have been solved, both for electrons and holes, the available information on energies and wave functions is used as input to calculate exciton energy and the effective band gap of the system. The lifetime of an exciton in a conical quantum dot has been estimated and shown to be in the range of nanoseconds. In addition, exciton-related Raman scattering, interband light absorption and photoluminescence in conical GaAs quantum dots have been calculated. It has been shown that with a decrease in the size of the quantum dot, the absorption peak has a blue shift, which is more pronounced for quantum dots of smaller sizes. Furthermore, the interband optical absorption and photoluminescence spectra have been revealed for different sizes of GaAs quantum dot.

Funder

European Union

Russian-Armenian University Development Program

Publisher

MDPI AG

Subject

General Materials Science,General Chemical Engineering

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