Combining Sun-Photometer, PM Monitor and SMPS to Inverse the Missing Columnar AVSD and Analyze Its Characteristics in Central China

Abstract

Columnar aerosol volume size distribution (AVSD) is an important atmospheric parameter that shows aerosol microphysical properties and can be used to analyze the impact of aerosols on the radiation budget balance, as well as regional climate effects. Usually, columnar AVSD can be obtained by using a sun photometer, but its observation conditions are relatively strict, and the columnar AVSD will be missing in cloudy or hazy weather due to cloud cover and other factors. This study introduces a novel algorithm for inversion of missing columnar AVSD under haze periods by using a machine learning approach and other ground-based observations. The principle is as follows. We are based on joint observational experiments. Since the scanning mobility particle sizer (SMPS) and particulate matter (PM) monitor sample the surface data, they can be stitched together to obtain the surface AVSD according to their observation range. Additionally, the sun-photometer scans the whole sky, so it can obtain columnar AVSD and aerosol optical depth (AOD). Then we use the back propagation neural network (BPNN) model to establish the relationship between the surface AVSD and the columnar AVSD and add AOD as a constraint. Next, the model is trained with the observation data of the same period. After the model training is completed, the surface AVSD and AOD can be used to invert the missing columnar AVSD during the haze period. In experiments on the 2015 dataset, the results show that the correlation coefficient and root mean square error between our model inversion results and the original sun photometer observations were 0.967 and 0.008 in winter, 0.968 and 0.010 in spring, 0.969 and 0.013 in summer, 0.972 and 0.007 in autumn, respectively. It shows a generally good performance that can be applied to the four seasons. Furthermore, the method was applied to fill the missing columnar AVSD of Wuhan, a city in central China, under adverse weather conditions. The final results were shown to be consistent with the climatic characteristics of Wuhan. Therefore, it can indeed solve the problem that sun photometer observations are heavily dependent on weather conditions, contributing to a more comprehensive study of the effects of aerosols on climate and radiation balance.