Highly Sensitive Pressure Sensor Based on Elastic Conductive Microspheres

Author:

Li Zhangling123,Guan Tong4,Zhang Wuxu123,Liu Jinyun123,Xiang Ziyin12ORCID,Gao Zhiyi12,He Jing5,Ding Jun6,Bian Baoru12,Yi Xiaohui12ORCID,Wu Yuanzhao12,Liu Yiwei12,Shang Jie12ORCID,Li Runwei12

Affiliation:

1. CAS Key Laboratory of Magnetic Materials and Devices, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo 315201, China

2. Zhejiang Province Key Laboratory of Magnetic Materials and Application Technology, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo 315201, China

3. College of Materials Science and Opto-Electronic Technology, University of Chinese Academy of Sciences, Beijing 100049, China

4. School of Materials Science and Engineering, Shanghai University, Shanghai 200072, China

5. School of Software and Electrical Engineering, Swinburne University of Technology, Melbourne 3122, Australia

6. Department of Materials Science and Engineering, National University of Singapore, Singapore 119260, Singapore

Abstract

Elastic pressure sensors play a crucial role in the digital economy, such as in health care systems and human–machine interfacing. However, the low sensitivity of these sensors restricts their further development and wider application prospects. This issue can be resolved by introducing microstructures in flexible pressure-sensitive materials as a common method to improve their sensitivity. However, complex processes limit such strategies. Herein, a cost-effective and simple process was developed for manufacturing surface microstructures of flexible pressure-sensitive films. The strategy involved the combination of MXene–single-walled carbon nanotubes (SWCNT) with mass-produced Polydimethylsiloxane (PDMS) microspheres to form advanced microstructures. Next, the conductive silica gel films with pitted microstructures were obtained through a 3D-printed mold as flexible electrodes, and assembled into flexible resistive pressure sensors. The sensor exhibited a sensitivity reaching 2.6 kPa−1 with a short response time of 56 ms and a detection limit of 5.1 Pa. The sensor also displayed good cyclic stability and time stability, offering promising features for human health monitoring applications.

Funder

National Natural Science Foundation of China

External Cooperation Program of Chinese Academy of Sciences

K.C. Wong Education Foundation

Chinese Academy of Sciences Youth Innovation Promotion Association

“Pioneer” and “Leading Goose” R&D Program of Zhejiang

Zhejiang Provincial Key R&D Program

“High-level talent special support plan” technology innovation leading talent project of Zhejiang Province

Natural Science Foundation of Zhejiang Province

Zhejiang Provincial Basic Public Welfare Research Project

Ningbo Scientific and Technological Innovation 2025 Major Project

China Postdoctoral Foundation

National Science Foundation of Ningbo

Publisher

MDPI AG

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