Observation of Dirac Charge-Density Waves in Bi2Te2Se

Abstract

While parallel segments in the Fermi level contours, often found at the surfaces of topological insulators (TIs), would imply “strong” nesting conditions, the existence of charge-density waves (CDWs)—periodic modulations of the electron density—has not been verified up to now. Here, we report the observation of a CDW at the surface of the TI Bi2Te2Se(111), below ≈350K, by helium-atom scattering and, thus, experimental evidence for a CDW involving Dirac topological electrons. Deviations of the order parameter observed below 180K, and a low-temperature break of time reversal symmetry, suggest the onset of a spin-density wave with the same period as the CDW in the presence of a prominent electron-phonon interaction, originating from Rashba spin-orbit coupling.