Visible Light‐Driven Hypochlorous Acid Synthesis Using a Sustainable and Cost‐Effective WO3/CdS Photocatalyst without Precious Metals

Author:

Wang Yi1ORCID,Han Shuiquan1,Lu Qingbiao1,Zhang Dun1,Wang Jin1,He Peng2

Affiliation:

1. Key Laboratory of Advanced Marine Materials Key Laboratory of Marine Environmental Corrosion and Bio-Fouling Institute of Oceanology Chinese Academy of Sciences Qingdao 266071 China

2. Wuhan Second Ship Design and Research Institute Wuhan 430205 China

Abstract

AbstractCompared with traditional electrolytic technology, directly using photocatalytic materials to produce hypochlorous acid from chlorine‐containing water undoubtedly has stronger low‐carbon and environmentally‐friendly characteristics. However, currently reported materials with photocatalytic chlorine production performance require precious metal Pt for catalysis, which undoubtedly greatly increases production costs. Therefore, developing new types of non‐precious metal‐based photocatalytic materials for efficient hypochlorous acid synthesis has significant implications. In this study, we demonstrate a novel breakthrough by showing that the WO3/CdS with a Z‐scheme structure effectively generated 3.54 mg/L of free chlorine in a 0.5 M NaCl solution, while also exhibiting spectral bactericidal and algal inhibition properties. The Z‐scheme structure can effectively prevent carrier recombination and improve photocatalytic efficiency. Therefore, this research provides a novel approach to photocatalytic antifouling and holds significant implications for the application of photocatalytic technology in the marine antifouling industry.

Publisher

Wiley

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