Impact of concentration and aging time of pea starch‐based polymeric solutions on the fabrication of electrospun nanofibers

Author:

da Cruz Elder Pacheco1ORCID,dos Santos Felipe Nardo1,de Souza Jaqueline Ferreira2,de Souza Estefania Júlia Dierings1,Fonseca Laura Martins1ORCID,Fajardo André Ricardo2,da Zavareze Elessandra Rosa1,Dias Alvaro Renato Guerra1

Affiliation:

1. Laboratory of Biopolymers and Nanotechnology in Food (BioNano), Graduate Program in Food Science and Technology, Department of Agroindustrial Science and Technology Federal University of Pelotas Pelotas RS Brazil

2. Laboratory of Technology and Development of Composites and Polymeric Materials (LaCoPol), Center for Chemical, Pharmaceutical and Food Sciences Federal University of Pelotas Pelotas RS Brazil

Abstract

AbstractPolymer concentration and aging time of polymeric solutions are crucial factors that can influence their viscosity, playing an essential role in the fabrication of electrospun nanofibers. Based on this, herein we evaluated the impact of aging time (24 and 48 h) and pea starch concentration (10%, 20%, and 30%, wt/vol) on the polymeric solutions to produce electrospun nanofibers. Solutions were evaluated by rheology, electrical conductivity, and degree of substitution. The nanofibers were analyzed by morphology, size distribution, chemical nature, and thermal properties. The degree of substitution of starches varied from 1.17 to 1.56. Overall, electrical conductivity decreased with increasing starch concentration and aging time of the polymeric solutions. The use of 10% starch displayed a transition from capsules to fibers, while 20% and 30% starch were able to manufacture homogenous, cylindrical, and random nanofibers with diameters varying from 89 to 373 nm. A significant impact of viscosity was not observed; on the other hand, aging time increased the average diameter of nanofibers. Besides, the fabricated nanofibers showed a lower decomposition temperature than raw starch. The fabricated nanofibers have great potential as wall materials for the encapsulation of different compounds and applications in the biomedical and food sectors.

Funder

Coordenação de Aperfeiçoamento de Pessoal de Nível Superior

Fundação de Amparo à Pesquisa do Estado do Rio Grande do Sul

Conselho Nacional de Desenvolvimento Científico e Tecnológico

Publisher

Wiley

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