Synthesis of Ferrocenyl Boranes and their Application as Lewis Acids in Epoxide Rearrangements

Author:

Köring Laura1,Birenheide Bernhard2,Krämer Felix2ORCID,Wenzel Jonas O.2ORCID,Schoch Roland1ORCID,Brehm Martin1ORCID,Breher Frank2ORCID,Paradies Jan1ORCID

Affiliation:

1. Chemistry Department Paderborn University Warburger Strasse 100 33098 Paderborn Germany

2. Institute of Inorganic Chemistry Karlsruhe Institute of Technology (KIT) Engesserstraße 15 76131 Karlsruhe Germany

Abstract

AbstractA series of substituted ferrocenyl boron derivatives was synthesized. The oxidation of the ferrocenyl unit resulted in a significant increase of the boron‐centered Lewis acidity. The neutral and cationic Lewis acids were characterized by NMR spectroscopy, crystal structure analysis and by computational methods. The new Lewis acids were then applied in the Meinwald rearrangement of epoxides, predominantly furnishing aldehydes as the kinetic products.

Funder

Fonds der Chemischen Industrie

Universität Paderborn

Publisher

Wiley

Reference109 articles.

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