Quantum Enhanced Probes of Magnetic Circular Dichroism

Author:

Hua Chengyun1,Marvinney Claire E.2,Hong Seongjin3,Feldman Matthew2,Pai Yun‐Yi1,Chilcote Michael1,Rabinowitz Joshua4,Pooser Raphael C.2,Marino Alberto M.2,Lawrie Benjamin J.1ORCID

Affiliation:

1. Materials Science and Technology Division Oak Ridge National Laboratory Oak Ridge TN 37831 USA

2. Computational Sciences and Engineering Division Oak Ridge National Laboratory Oak Ridge TN 37831 USA

3. Physics Division Oak Ridge National Laboratory Oak Ridge TN 37831 USA

4. Department of Physics Duke University Durham NC 27708 USA

Abstract

AbstractMagneto‐optical microscopies, including optical measurements of magnetic circular dichroism, are increasingly ubiquitous tools for probing spin‐orbit coupling, charge‐carrier g‐factors, and chiral excitations in matter, but the minimum detectable signal in classical magnetic circular dichroism measurements is fundamentally limited by the shot‐noise limit of the optical readout field. Here, a two‐mode squeezed light source is used to improve the minimum detectable signal in magnetic circular dichroism measurements by 3 decibels compared with state‐of‐the‐art classical measurements, even with relatively lossy samples like terbium gallium garnet. These results provide a framework for new quantum‐enhanced magneto‐optical microscopies that are particularly critical for environmentally sensitive materials and for low temperature measurements where increased optical power can introduce unacceptable thermal perturbations.

Funder

Office of Science

Basic Energy Sciences

Publisher

Wiley

Subject

Electrical and Electronic Engineering,Computational Theory and Mathematics,Condensed Matter Physics,Mathematical Physics,Nuclear and High Energy Physics,Electronic, Optical and Magnetic Materials,Statistical and Nonlinear Physics

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