Photothermal‐Enhanced Uranium Extraction from Seawater: A Biomass Solar Thermal Collector with 3D Ion‐Transport Networks

Author:

Li Tingyang12,Lin Xiangbin12,Zhang Zhehua12,Yang Linsen1,Qian Yongchao1,Fu Lin12,Zhou Shengyang1,Chen Weipeng1,Wang Qingchen12,Li Xin12,Kong Xiang‐Yu12,Xiao Hongyan1,Jiang Lei12,Wen Liping12ORCID

Affiliation:

1. CAS Key Laboratory of Bio‐inspired Materials and Interfacial Science Technical Institute of Physics and Chemistry Department Chinese Academy of Sciences Beijing 100190 P. R. China

2. School of Future Technology University of Chinese Academy of Sciences Beijing 9100049 P. R. China

Abstract

AbstractAccess to uranium resources is critical to the sustainable development of nuclear energy. The ocean contains abundant uranium resources, but the marine biological pollution and the low concentration of uranium make it a giant challenge to extract uranium from seawater. On the foundation of selective uranium adsorption using high uranium‐affinity groups, realizing the external‐field improved uranium capture without extra energy consumption is highly attractive. A solar thermal collector with 3D ion‐transport networks based on environmentally friendly biomass adsorption material is reported, which contains antibacterial adsorption ligands and photothermal graphene oxide. The antibacterial ability through an easy one‐step reaction and the fast mass transfer caused by photothermal conversion collaboratively improve the original adsorption capacity of the hydrogel by 46.7%, reaching 9.18 mg g−1 after contact with natural seawater for 14 days. This study provides a universal strategy for the design of physical‐fields‐enhanced hydrogel adsorbents.

Publisher

Wiley

Subject

Electrochemistry,Condensed Matter Physics,Biomaterials,Electronic, Optical and Magnetic Materials

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