2D Metal Phosphorous Trichalcogenides (MPCh3) for Sustainable Energy Storage and Conversion: Nanoarchitectonics and Advanced Applications

Author:

Wang Honglei1,Cheng Pengfei1,Wu Bing2,Yan Yong3,Schaaf Peter1,Sofer Zdenek2,Wang Dong1ORCID

Affiliation:

1. Chair Materials for Electrical Engineering and Electronics Institute of Materials Science and Engineering and Institute of Micro and Nanotechnologies MacroNano TU Ilmenau, Gustav‐Kirchhoff‐Str. 5 98693 Ilmenau Germany

2. Department of Inorganic Chemistry University of Chemistry and Technology Prague Technická 5 Prague 6 166 28 Czech Republic

3. Center of Excellence for Environmental Safety and Biological Effects Beijing Key Laboratory for Green Catalysis and Separation Department of Chemistry Beijing University of Technology Beijing 100124 China

Abstract

Abstract2D metal phosphorous trichalcogenides (MPCh3) have attracted considerable attention in sustainable energy storage and conversion due to their distinct physical and chemical characteristics, such as adjustable energy bandgap, significant specific surface area, and abundant active sites. However, research on 2D MPCh3 primarily focuses on electrocatalysis, and understanding its energy conversion and storage mechanisms remains incomplete. This review comprehensively summarizes recent advancements in energy storage and conversion using 2D MPCh3‐based materials of various structures. It begins with a discussion of the distinctive properties and preparation techniques of 2D MPCh3, followed by a focus on the rational design and development of these materials for diverse energy‐related applications, including rechargeable batteries, supercapacitors, electrocatalysis, photocatalysis, and desalination. Finally, it outlines the key challenges and prospects for future research on 2D MPCh3 materials.

Funder

China Scholarship Council

National Natural Science Foundation of China

Publisher

Wiley

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