Electric Field‐Manipulated Optical Chirality in Ferroelectric Vortex Domains

Author:

Han Haojie1,Li Wei1,Zhang Qinghua2,Tang Shiyu3,Wang Yue1,Xu Zongqi1,Liu Yiqun1,Chen Hetian1,Gu Jingkun1,Wang Jing3,Yi Di1,Gu Lin1,Huang Houbing3,Nan Ce‐Wen1,Li Qian1ORCID,Ma Jing1ORCID

Affiliation:

1. State Key Laboratory of New Ceramics and Fine Processing School of Materials Science and Engineering Tsinghua University Beijing 100084 China

2. Beijing National Laboratory for Condensed Matter Physics Institute of Physics Chinese Academy of Science Beijing 100190 China

3. Advanced Research Institute of Multidisciplinary Science, and School of Materials Science and Engineering Beijing Institute of Technology Beijing 100081 China

Abstract

AbstractManipulating optical chirality via electric fields has garnered considerable attention in the realm of both fundamental physics and practical applications. Chiral ferroelectrics, characterized by their inherent optical chirality and switchable spontaneous polarization, are emerging as a promising platform for electronic‐photonic integrated circuits applications. Unlike organics with chiral carbon centers, integrating chirality into technologically mature inorganic ferroelectrics has posed a long‐standing challenge. Here, the successful introduction of chirality is reported into self‐assembly La‐doped BiFeO3 nanoislands, which exhibit ferroelectric vortex domains. By employing synergistic experimental techniques with piezoresponse force microscopy and nonlinear optical second‐harmonic generation probes, a clear correlation between chirality and polarization configuration within these ferroelectric nanoislands is established. Furthermore, the deterministic control of ferroelectric vortex domains and chirality is demonstrated by applying electric fields, enabling reversible and nonvolatile generation and elimination of optically chiral signals. These findings significantly expand the repertoire of field‐controllable chiral systems and lay the groundwork for the development of innovative ferroelectric optoelectronic devices.

Funder

National Natural Science Foundation of China

National Key Research and Development Program of China

Publisher

Wiley

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