Novel quantification of regional fossil fuel CO 2 reductions during COVID-19 lockdowns using atmospheric oxygen measurements

Author:

Pickers Penelope A.1ORCID,Manning Andrew C.1ORCID,Le Quéré Corinne1ORCID,Forster Grant L.12ORCID,Luijkx Ingrid T.3ORCID,Gerbig Christoph4ORCID,Fleming Leigh S.1ORCID,Sturges William T.1ORCID

Affiliation:

1. Centre for Ocean and Atmospheric Sciences, School of Environmental Sciences, University of East Anglia, Norwich NR4 7TJ, UK.

2. National Centre for Atmospheric Science, University of East Anglia, Norwich NR4 7TJ, UK.

3. Department of Meteorology and Air Quality, Wageningen University and Research, 6700AA Wageningen, the Netherlands.

4. Department of Biogeochemical Systems, Max Planck Institute for Biogeochemistry, Jena, Germany.

Abstract

It is not currently possible to quantify regional-scale fossil fuel carbon dioxide (ffCO 2 ) emissions with high accuracy in near real time. Existing atmospheric methods for separating ffCO 2 from large natural carbon dioxide variations are constrained by sampling limitations, so that estimates of regional changes in ffCO 2 emissions, such as those occurring in response to coronavirus disease 2019 (COVID-19) lockdowns, rely on indirect activity data. We present a method for quantifying regional signals of ffCO 2 based on continuous atmospheric measurements of oxygen and carbon dioxide combined into the tracer “atmospheric potential oxygen” (APO). We detect and quantify ffCO 2 reductions during 2020–2021 caused by the two U.K. COVID-19 lockdowns individually using APO data from Weybourne Atmospheric Observatory in the United Kingdom and a machine learning algorithm. Our APO-based assessment has near–real-time potential and provides high-frequency information that is in good agreement with the spread of ffCO 2 emissions reductions from three independent lower-frequency U.K. estimates.

Publisher

American Association for the Advancement of Science (AAAS)

Subject

Multidisciplinary

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