A scalable metal-organic framework as a durable physisorbent for carbon dioxide capture-Reference-Cited by-同舟云学术

A scalable metal-organic framework as a durable physisorbent for carbon dioxide capture

Published:2021-12-17 Issue:6574 Volume:374 Page:1464-1469
ISSN:0036-8075
Container-title:Science
language:en
Short-container-title:Science

Author:

Lin Jian-Bin¹^ORCID,Nguyen Tai T. T.²^ORCID,Vaidhyanathan Ramanathan¹³^ORCID,Burner Jake⁴^ORCID,Taylor Jared M.¹⁵,Durekova Hana⁴,Akhtar Farid⁶^ORCID,Mah Roger K.¹⁵,Ghaffari-Nik Omid⁷^ORCID,Marx Stefan⁸^ORCID,Fylstra Nicholas¹^ORCID,Iremonger Simon S.¹,Dawson Karl W.¹,Sarkar Partha²^ORCID,Hovington Pierre⁷^ORCID,Rajendran Arvind²^ORCID,Woo Tom K.⁴^ORCID,Shimizu George K. H.¹⁵^ORCID

Affiliation:

1. Department of Chemistry, University of Calgary, Calgary, Alberta, Canada.

2. Department of Chemical and Materials Engineering, University of Alberta, Edmonton, Alberta, Canada.

3. Indian Institute of Science Education and Research, Dr. Homi Bhabha Road, Pashan, Pune, Maharashtra, 411008, India.

4. Department of Chemistry and Biomolecular Science, University of Ottawa, Ottawa, Ontario, Canada.

5. ZoraMat Solutions Inc., Calgary, Alberta, Canada.

6. Department of Materials Engineering, Luleå University of Technology, Luleå, Sweden.

7. Svante Inc., Vancouver, British Columbia, Canada.

8. BASF SE, Ludwigshafen am Rhein, Germany.

Abstract

A hydrophobic CO 2 physisorbent Most materials for carbon dioxide (CO 2 ) capture of fossil fuel combustion, such as amines, rely on strong chemisorption interactions that are highly selective but can incur a large energy penalty to release CO 2 . Lin et al . show that a zinc-based metal organic framework material can physisorb CO 2 and incurs a lower regeneration penalty. Its binding site at the center of the pores precludes the formation of hydrogen-bonding networks between water molecules. This durable material can preferentially adsorb CO2 at 40% relative humidity and maintains its performance under flue gas conditions of 150°C. —PDS

Publisher

American Association for the Advancement of Science (AAAS)

Subject

Multidisciplinary

Reference74 articles.

1. “Accelerating Breakthrough Innovation in Carbon Capture Utilization and Storage” (U.S. Department of Energy 2017).

2. CO2 Capture in Metal-Organic Framework Adsorbents: An Engineering Perspective

3. Carbon Dioxide Capture in Metal–Organic Frameworks

4. Amine-Based CO2 Capture Technology Development from the Beginning of 2013—A Review

5. Process intensification for post-combustion CO2 capture with chemical absorption: A critical review

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