Hidden order in spin-liquid Gd 3 Ga 5 O 12

Author:

Paddison Joseph A. M.123,Jacobsen Henrik45,Petrenko Oleg A.6,Fernández-Díaz Maria Teresa7,Deen Pascale P.45,Goodwin Andrew L.1

Affiliation:

1. Department of Chemistry, University of Oxford, Inorganic Chemistry Laboratory, South Parks Road, Oxford OX1 3QR, UK.

2. ISIS Facility, Rutherford Appleton Laboratory, Chilton, Didcot, Oxfordshire OX11 0QX, UK.

3. School of Physics, Georgia Institute of Technology, Atlanta, GA 30332, USA.

4. Nanoscience Center, Niels Bohr Institute, University of Copenhagen, DK-2100 Copenhagen Ø, Denmark.

5. European Spallation Source, Tunavägen 24, Lund, Sweden.

6. Department of Physics, University of Warwick, Coventry, CV4 7AL, UK.

7. Institut Max von Laue–Paul Langevin, F-38042 Grenoble 9, France.

Abstract

Elucidating order within disorder In some materials, the geometry of the crystal lattice gets in the way of magnetic ordering. Their spins, although magnetically interacting, remain seemingly disordered and form a so-called spin liquid. Paddison et al. propose a different model for the spin-liquid compound Gd 3 Ga 5 O 12 . Neutron diffraction measurements and numerical techniques revealed that even though individual spins in this material were disordered, they formed 10-spin loops that were correlated with one another. The nature of this “hidden order” was such that it escaped direct detection by conventional techniques Science , this issue p. 179

Funder

ERC

EPSRC

STFC

Danish Research Council for Nature and Universe

Publisher

American Association for the Advancement of Science (AAAS)

Subject

Multidisciplinary

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