Direct Observations of Atmospheric Aerosol Nucleation

Author:

Kulmala Markku1,Kontkanen Jenni1,Junninen Heikki1,Lehtipalo Katrianne1,Manninen Hanna E.1,Nieminen Tuomo12,Petäjä Tuukka1,Sipilä Mikko1,Schobesberger Siegfried1,Rantala Pekka1,Franchin Alessandro1,Jokinen Tuija1,Järvinen Emma1,Äijälä Mikko1,Kangasluoma Juha1,Hakala Jani1,Aalto Pasi P.1,Paasonen Pauli1,Mikkilä Jyri3,Vanhanen Joonas3,Aalto Juho4,Hakola Hannele5,Makkonen Ulla5,Ruuskanen Taina1,Mauldin Roy L.16,Duplissy Jonathan1,Vehkamäki Hanna1,Bäck Jaana7,Kortelainen Aki8,Riipinen Ilona9,Kurtén Theo110,Johnston Murray V.11,Smith James N.812,Ehn Mikael113,Mentel Thomas F.13,Lehtinen Kari E. J.58,Laaksonen Ari58,Kerminen Veli-Matti1,Worsnop Douglas R.15814

Affiliation:

1. Department of Physics, University of Helsinki, Finland.

2. Helsinki Institute of Physics, Helsinki, Finland.

3. Airmodus Oy, Helsinki, Finland.

4. SMEAR Station II, Hyytiälä, Finland.

5. Finnish Meteorological Institute, Finland.

6. University of Colorado at Boulder, Boulder, CO, USA.

7. Department of Forest Sciences, University of Helsinki, Finland.

8. University of Eastern Finland, Kuopio, Finland.

9. University of Stockholm, Stockholm, Sweden.

10. Department of Chemistry, University of Helsinki, Finland.

11. University of Delaware, Newark, DE, USA.

12. National Center for Atmospheric Research, Boulder, CO, USA.

13. Forschungszentrum Juelich, IEK-8, 52425 Juelich, Germany.

14. Aerodyne Research, Billerica, MA, USA.

Abstract

Aerosol Formation Most atmospheric aerosol particles result from a growth process that begins with atmospheric molecules and clusters, progressing to larger and larger sizes as they acquire other molecules, clusters, and particles. The initial steps of this process involve very small entities—with diameters of less than 2 nanometers—which have been difficult to observe. Kulmala et al. (p. 943 ; see the Perspective by Andreae ) developed a sensitive observational protocol that allows these tiny seeds to be detected and counted, and they mapped out the process of aerosol formation in detail.

Publisher

American Association for the Advancement of Science (AAAS)

Subject

Multidisciplinary

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