Atomic-scale spin sensing with a single molecule at the apex of a scanning tunneling microscope

Author:

Verlhac B.1ORCID,Bachellier N.1,Garnier L.1,Ormaza M.1ORCID,Abufager P.2,Robles R.3ORCID,Bocquet M.-L.4ORCID,Ternes M.56ORCID,Lorente N.37ORCID,Limot L.1ORCID

Affiliation:

1. Université de Strasbourg, CNRS, IPCMS, UMR 7504, F-67000 Strasbourg, France.

2. Instituto de Física de Rosario, CONICET and Universidad Nacional de Rosario, Av. Pellegrini 250 (2000) Rosario, Argentina.

3. Centro de Física de Materiales CFM/MPC (CSIC-UPV/EHU), 20018 Donostia-San Sebastián, Spain.

4. PASTEUR, Département de Chimie, Ecole Normale Supérieure, PSL Research University, Sorbonne Universités, UPMC Univ. Paris 06, CNRS, 75005 Paris, France.

5. Institute of Physics II B, RWTH Aachen University, 52074 Aachen, Germany.

6. Peter Grünberg Institut (PGI-3), Forschungszentrum Jülich, 52425 Jülich, Germany.

7. Donostia International Physics Center (DIPC), 20018 Donostia-San Sebastián, Spain.

Abstract

Single molecules sense spin Imaging surface magnetism, and, in particular, spin excitations of adsorbed molecules or films, is challenging. Verlhac et al. demonstrate spin-sensing capability by using the magnetic exchange interaction between a surface sample and the spin-excited states of a nickelocene molecule attached to a scanning tunneling microscope tip. The spatial dependence of the exchange field at the atomic scale enabled imaging of magnetic corrugation with atomic-scale lateral resolution for iron atoms and small islands of cobalt atoms absorbed on nonmagnetic copper surfaces. Science , this issue p. 623

Funder

Ministerio de Ciencia, Innovación y Universidades

European Commission

Deutsche Forschungsgemeinschaft

Agence Nationale de la Recherche

Publisher

American Association for the Advancement of Science (AAAS)

Subject

Multidisciplinary

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