Magnetic hysteresis up to 80 kelvin in a dysprosium metallocene single-molecule magnet

Author:

Guo Fu-Sheng1ORCID,Day Benjamin M.12ORCID,Chen Yan-Cong3ORCID,Tong Ming-Liang3ORCID,Mansikkamäki Akseli4ORCID,Layfield Richard A.1ORCID

Affiliation:

1. Department of Chemistry, School of Life Sciences, University of Sussex, Falmer BN1 9QJ, UK.

2. School of Chemistry, The University of Manchester, Oxford Road, Manchester M13 9PL, UK.

3. Key Laboratory of Bioinorganic and Synthetic Chemistry of the Ministry of Education, School of Chemistry, Sun-Yat Sen University, Guangzhou 510275, People’s Republic of China.

4. Department of Chemistry, Nanoscience Centre, University of Jyväskylä, P.O. Box 35, FI-40014 Jyväskylä, Finland.

Abstract

Breaking through the nitrogen ceiling Single-molecule magnets could prove useful in miniaturizing a wide variety of devices. However, their application has been severely hindered by the need to cool them to extremely low temperature using liquid helium. Guo et al. now report a dysprosium compound that manifests magnetic hysteresis at temperatures up to 80 kelvin. The principles applied to tuning the ligands in this complex could point the way toward future architectures with even higher temperature performance. Science , this issue p. 1400

Funder

H2020 European Research Council

Engineering and Physical Sciences Research Council

Publisher

American Association for the Advancement of Science (AAAS)

Subject

Multidisciplinary

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