Remnants of the Early Solar System Water Enriched in Heavy Oxygen Isotopes

Author:

Sakamoto Naoya1234,Seto Yusuke1234,Itoh Shoichi1234,Kuramoto Kiyoshi1234,Fujino Kiyoshi1234,Nagashima Kazuhide1234,Krot Alexander N.1234,Yurimoto Hisayoshi1234

Affiliation:

1. Department of Natural History Sciences, Hokkaido University, Sapporo 060-0810, Japan.

2. Department of Cosmosciences, Hokkaido University, Sapporo 060-0810, Japan.

3. Hawai'i Institute of Geophysics and Planetology, School of Ocean and Earth Science and Technology, University of Hawai'i at Manoa, Honolulu, HI 96822, USA.

4. Isotope Imaging Laboratory, Creative Research Initiative “Sousei,” Hokkaido University, Sapporo, 001-0021, Japan.

Abstract

Oxygen isotopic composition of our solar system is believed to have resulted from mixing of two isotopically distinct nebular reservoirs, 16 O-rich and 17,18 O-rich relative to Earth. The nature and composition of the 17,18 O-rich reservoir are poorly constrained. We report an in situ discovery of a chemically and isotopically unique material distributed ubiquitously in fine-grained matrix of a primitive carbonaceous chondrite Acfer 094. This material formed by oxidation of Fe,Ni-metal and sulfides by water either in the solar nebula or on a planetesimal. Oxygen isotopic composition of this material indicates that the water was highly enriched in 17 O and 18 O (δ 17,18 O SMOW = +180‰ per mil), providing the first evidence for an extremely 17,18 O-rich reservoir in the early solar system.

Publisher

American Association for the Advancement of Science (AAAS)

Subject

Multidisciplinary

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