Precise pitch-scaling of carbon nanotube arrays within three-dimensional DNA nanotrenches

Author:

Sun Wei12ORCID,Shen Jie12ORCID,Zhao Zhao134,Arellano Noel5,Rettner Charles5,Tang Jianshi6ORCID,Cao Tianyang1ORCID,Zhou Zhiyu1ORCID,Ta Toan5ORCID,Streit Jason K.7ORCID,Fagan Jeffrey A.7ORCID,Schaus Thomas12ORCID,Zheng Ming7,Han Shu-Jen6,Shih William M.134,Maune Hareem T.5ORCID,Yin Peng12ORCID

Affiliation:

1. Wyss Institute for Biologically Inspired Engineering, Harvard University, Boston, MA 02115, USA.

2. Department of Systems Biology, Harvard Medical School, Boston, MA 02115, USA.

3. Department of Cancer Biology, Dana-Farber Cancer Institute, Harvard Medical School, Boston, MA 02115, USA.

4. Department of Biological Chemistry and Molecular Pharmacology, Harvard Medical School, Boston, MA 02115, USA.

5. IBM Almaden Research Center, San Jose, CA 95120, USA.

6. IBM Thomas J. Watson Research Center, Yorktown Heights, NY 10598, USA.

7. Materials Science and Engineering Division, National Institute of Standards and Technology (NIST), Gaithersburg, MD 20899, USA.

Abstract

DNA bricks build nanotube transistors Semiconducting carbon nanotubes (CNTs) are an attractive platform for field-effect transistors (FETs) because they potentially can outperform silicon as dimensions shrink. Challenges to achieving superior performance include creating highly aligned and dense arrays of nanotubes as well as removing coatings that increase contact resistance. Sun et al. aligned CNTs by wrapping them with single-stranded DNA handles and binding them into DNA origami bricks that formed an array of channels with precise intertube pitches as small as 10.4 nanometers. Zhao et al. then constructed single and multichannel FETs by attaching the arrays to a polymer-templated silicon wafer. After adding metal contacts across the CNTs to fix them to the substrate, they washed away all of the DNA and then deposited electrodes and gate dielectrics. The FETs showed high on-state performance and fast on-off switching. Science , this issue p. 874 , p. 878

Funder

National Science Foundation

Office of Naval Research

NIH Office of the Director

Air Force Office of Scientific Research

Publisher

American Association for the Advancement of Science (AAAS)

Subject

Multidisciplinary

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