Imaging the short-lived hydroxyl-hydronium pair in ionized liquid water-Reference-Cited by-同舟云学术

Imaging the short-lived hydroxyl-hydronium pair in ionized liquid water

Published:2021-10 Issue:6563 Volume:374 Page:92-95
ISSN:0036-8075
Container-title:Science
language:en
Short-container-title:Science

Author:

Lin M.-F.¹^ORCID,Singh N.²^ORCID,Liang S.³,Mo M.¹^ORCID,Nunes J. P. F.⁴^ORCID,Ledbetter K.⁵⁶^ORCID,Yang J.¹⁵^ORCID,Kozina M.¹^ORCID,Weathersby S.¹^ORCID,Shen X.¹^ORCID,Cordones A. A.⁵^ORCID,Wolf T. J. A.¹⁵^ORCID,Pemmaraju C. D.⁷^ORCID,Ihme M.²^ORCID,Wang X. J.¹^ORCID

Affiliation:

1. SLAC National Accelerator Laboratory, Menlo Park, CA 94025, USA.

2. Department of Mechanical Engineering, Stanford University , Stanford, CA 94305, USA.

3. Department of Chemistry, Stanford University, Stanford, CA 94305, USA.

4. Department of Physics and Astronomy, University of Nebraska–Lincoln, Lincoln, NE 68588, USA.

5. Stanford PULSE Institute, SLAC National Accelerator Laboratory, Menlo Park, CA 94025, USA.

6. Department of Physics, Stanford University, Stanford, CA 94305, USA.

7. SIMES, SLAC National Accelerator Laboratory, Menlo Park, CA 94025, USA.

Abstract

Capturing OH(H 3 O + ) in ionized water Recent advances in liquid-phase ultrafast electron diffraction techniques make it possible to observe what has only been theoretically presumed to occur at short times upon interaction of ionizing radiation with liquid water. Lin et al . provide direct evidence for capturing the short-lived radical-cation pair OH(H 3 O + ), which has been hypothesized for years to form after ionization of liquid water but was not structurally resolved previously (see the Perspective by Cao et al .). The authors trace dissociation and subsequent nonradiative structural relaxation around the ionization center. —YS

Publisher

American Association for the Advancement of Science (AAAS)

Subject

Multidisciplinary

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