Novel Role of Molecular Perovskite Energetic Materials: A Potential High-Energy Oxidant for the Solid Rocket Propellant

Author:

Peng Deng,Guo Xueyong,Fang Hua,Liu Rui,Chen Pengwan

Publisher

Elsevier BV

Subject

General Earth and Planetary Sciences,General Environmental Science

Reference51 articles.

1. As shown in Fig. 5, the melting endothermic peak of raw Al was located at 656 �C. For the mixed powders DAP-4/Al or composites DAP-4/Al/F, DAP-4 molecules with rich ClO 4 -anion was easy to be ignited at the first stage [6,24], to release strong acid and oxidizing gas as well as a lot of energy. As shown in Fig. 8a, the maximum flame temperature of raw DAP-4 are up to 1065 �C. Acid gases, such as HCl, can directly corrode Al 2 O 3 shells on Al particle surfaces under a lower high-temperature environment, which improved ignition performance of Al at the ensuing second stage, and oxidizing gas ( � O 2 -) also can directly act on Al with melting state through the Al 2 O 3 shell. As a result, the contents of HCl and Cl -anion had been reduced during the pyrolysis process at the pyrolysis temperature of 400 �C in Fig. 13 b and c. This will accelerate the combustion reaction of DAP-4/Al. A lot of energy from the self combustion of DAP-4 can enhanced overall combustion performances of DAP-4/Al;The metal fuel Al particles started the ignition and combustion reaction mainly depended on more energy released by DAP-4 thermal decomposition and combustion reaction at the last stage

2. Molecular perovskite high-energetic materials;S Chen;Sci. China Mater,2018

3. Optimizing the oxygen balance by changing the A-site cations in molecular perovskite high-energetic materials;S Chen;CrystEngComm,2018

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5. Metal-Free Hexagonal Perovskite High-Energetic Materials with NH 3 OH + /NH 2 NH 3 + as B-Site Cations;Y Shang;Engineering,2020

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