Abstract
Abstract
The effect of negative chemical pressure with the substitution of transition metal V in an itinerant helimagnetically ordered MnSi, Mn
1
−
x
V
x
Si with x = 0–0.1, is explored using dc and ac-susceptibilities. With increasing x, the manifestations are unaffected crystal structure with increasing unit cell volume, suppression of long-range magnetic order, weakening of itinerant character and reduced spin-cooperative phenomenon. The emergence of spin-glass behaviour for
x
⩾
0.1
intervenes in the occurrence of quantum phase transition. The constructed concentration-temperature x-T phase diagram illustrates the substitution-driven changes in the magnetism of MnSi. Further, the study suggests that the presence of a precursor state can favour the formation of spin-textures in magnetically ordered compositions
0
<
x
⩽
0.05
below the ordering temperature.
Funder
Science and Engineering Research Board