Van Hove singularity driven enhancement of superconductivity in two-dimensional tungsten monofluoride (WF)

Author:

Jamwal Prarena,Ahuja RajeevORCID,Kumar RakeshORCID

Abstract

Abstract Superconductivity in two-dimensional materials has gained significant attention in the last few years. In this work, we report phonon-mediated superconductivity investigations in monolayer Tungsten monofluoride (WF) by solving anisotropic Migdal Eliashberg equations as implemented in EPW. By employing first-principles calculations, our examination of phonon dispersion spectra suggests that WF is dynamically stable. Our results show that WF has weak electron–phonon coupling (EPC) strength (λ) of 0.49 with superconducting transition temperature (T c ) of 2.6 K. A saddle point is observed at 0.11 eV below the Fermi level (E F ) of WF, which corresponds to the Van Hove singularity (VHS). On shifting the Fermi level to the VHS by hole doping (3.7 × 1014 cm−2), the EPC strength increases to 0.93, which leads to an increase in the T c to 11 K. However, the superconducting transition temperature of both pristine and doped WF increases to approximately 7.2 K and 17.2 K, respectively, by applying the Full Bandwidth (FBW) anisotropic Migdal–Eliashberg equations. Our results provide a platform for the experimental realization of superconductivity in WF and enhancement of the superconducting transition temperature by adjusting the position of E F to the VHS.

Publisher

IOP Publishing

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