Abstract
The strong coupling of atoms and molecules to radiation field modes in optical cavities creates dressed matter/field states known as polaritons with controllable dynamical and energy transfer properties. We propose a multidimensional optical spectroscopy technique for monitoring polariton dynamics. The response of a two-level atom to the time-dependent coupling to a single-cavity mode is monitored through time-and-frequency–resolved single-photon coincidence measurements of spontaneous emission. Polariton population and coherence dynamics and its variation with cavity photon number and controlled by gating parameters are predicted by solving the Jaynes–Cummings model.
Funder
National Science Foundation
U.S. Department of Energy
Zijiang Endowed Young Scholar Fund
Publisher
Proceedings of the National Academy of Sciences
Cited by
24 articles.
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