Conceptual design of a fixed bed N2O decomposition reactor with a heat pipe heat exchanger
Author:
He Dong1, Bai Xiaoyue1, Tao Hanzhong1, Li Yannan1, Lin Shuo1
Affiliation:
1. College of Energy Science and Engineering , 506244 Nanjing Tech University , Nanjing , Jiangsu 211800 , China
Abstract
Abstract
This paper introduces a novel process for decomposing N2O through interstage cooling utilizing a heat pipe heat exchanger. The reactor design involves segmenting the fixed bed reactor into multiple layers and integrating heat pipe heat exchangers between these layers to efficiently dissipate the high heat generated by the upper fixed bed reactor. This innovative approach facilitates the direct decomposition of N2O feedgas with high concentrations, obviating the need for gas dilution. The study conducted in this paper employed Fluent and ASPEN PLUS to investigate N2O decomposition with interstage cooling using heat pipe heat exchangers, as well as decomposition after dilution. A comparison between the two methods was made based on catalyst dosage, temperature uniformity, and reactor energy consumption. The results demonstrate that the proposed method for N2O decomposition via interstage cooling with a heat pipe heat exchanger is a viable option, offering the desired temperature control and enhanced efficiency. Furthermore, this reactor design effectively reduces both catalyst usage and energy consumption, providing substantial advantages over traditional approaches.
Publisher
Walter de Gruyter GmbH
Reference27 articles.
1. K Protocol, Kyoto Protocol. UNFCCC Website, 1997. Available at: http://unfccc.int/kyoto_protocol/items/2830.php Accessed: Jan. 1, 2011. 2. M Protocol, Montreal Protocol on Substances that Deplete the Ozone Layer, vol. 26, Washington, DC, US Government Printing Office, 1987, pp. 128–136. 3. Y. Yung, W. Wang, and A. Lacis, “Greenhouse effect due to atmospheric nitrous oxide,” Geophys. Res. Lett., vol. 3, no. 10, pp. 619–621, 1976, https://doi.org/10.1029/gl003i010p00619. 4. A. Shimizu, K. Tanaka, and M. Fujimori, “Abatement technologies for N2O emissions in the adipic acid industry,” Chemosphere Global Change Sci., vol. 2, nos. 3–4, pp. 425–434, 2000, https://doi.org/10.1016/s1465-9972(00)00024-6. 5. J. Pérez-Ramı́rez, F. Kapteijn, G. Mul, X. Xu, and J. A. Moulijn, “Ex-framework FeZSM-5 for control of N2O in tail-gases,” Catal. Today, vol. 76, no. 1, pp. 55–74, 2002, https://doi.org/10.1016/s0920-5861(02)00208-0.
|
|