Abstract
AbstractThe k0 values of 6 non-1/v nuclides (152Eu, 152mEu, 154Eu, 177Lu, 192Ir and 194Ir) were determined using the extended Høgdahl formalism at the research reactor FRM II with very high f values. Standards were irradiated in 4 channels at different local temperatures between 40 °C and 55 °C measured using temperature sensitive irreversible labels. A good agreement with the recommended values was found for 152Eu, 154Eu and 177Lu using the original g(Tn) factors by Gryntakis, however, the k0 values for 152mEu in this work were 7% higher. New k0 values were also determined using the g(Tn) factors by Van Sluijs. Differences up to 6% were found for Eu isotopes compared with the recommended values. The recommended k0 values for 192Ir and 194Ir could be confirmed using g = 1. The theoretical k0 values for 177Lu were calculated using new nuclear data. They are up to 6% less than the recommended values. The present k0 values determined in this work showed a similar trend. The influence of different g(Tn) factors on the determination of the k0 values was investigated.
Funder
Technische Universität München
Publisher
Springer Science and Business Media LLC
Subject
Health, Toxicology and Mutagenesis,Public Health, Environmental and Occupational Health,Spectroscopy,Pollution,Radiology, Nuclear Medicine and imaging,Nuclear Energy and Engineering,Analytical Chemistry
Reference27 articles.
1. Høgdahl O.T (1962) Neutron absorption in pile neutron activation analysis, Report MMPP-226–1
2. De Corte F (1987) The k0-standardization method: a move to the optimization of neutron activation analysis. Habil. Thesis, University of Gent, Belgium
3. Westcott CH (1960) Effective cross section values for well-moderated thermal reactor spectra, report CRRP-960 of the AECL-1101, Nov. 1, 1960 (reprinted 1970)
4. De Corte F, Simonits A, Bellemans F, Freitas MC, Jovanović S, Smodiš B, Erdmann G, Petri H, De Wispelaere A (1993) Recent advances in the k0-standardization of neutron activation analysis: Extensions, applications, prospects. J Radioanal Nucl Chem 169:125–158
5. De Corte F, Bellemans F, De Neve P, Simonits A (1994) The use of a modified Westcott-formalism in the k0-standardization of NAA: The state of affairs. J Radioanal Nucl Chem 179:93–103
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